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I'm not sure about 9.1 but in 9.2 you can add new material in following way:
select 3D Modeller -> Assign Material -> Add Material
You should check at least relative permittivity property, probably also dielectric loss tangent. Other properties are relative permeability, conductivity and magnetic loss tangent. Magnetic saturation, Lande G Factor and Delta H are ferrite properties.
Search from Help -> Contents"adding new material", you'll find more explanations from there.
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